Accurate Representations of the Physicochemical Properties of Atmospheric Aerosols::  When are Laboratory Measurements of Value?

Aleksandra Marsh; Grazia Rovelli; Young-Chul Song; Kelly Louise Pereira; Rose Willoughby; Bryan Bzdek; Jacqueline Fiona Hamilton; andrew Orr-Ewing; David Topping; Reid Jonathan

doi:10.1039/C7FD00008A

Accurate Representations of the Physicochemical Properties of Atmospheric Aerosols: When are Laboratory Measurements of Value?

Aleksandra Marsh, Grazia Rovelli, Young-Chul Song, Kelly Louise Pereira, Rose Willoughby, Bryan Bzdek, Jacqueline Fiona Hamilton, andrew Orr-Ewing, David Topping, Reid Jonathan

Chemistry

Research output: Contribution to journal › Article › peer-review

Abstract

Laboratory studies can provide important insights into the processes that occur at the mesoscale in ambient aerosol. We examine the accuracies of measurements of core physicochemical properties of aerosols that can be made in single particle studies and explore the impact of these properties on the microscopic processes that occur in ambient aerosol. Presenting new measurements, we examine here the refinements in our understanding of aerosol hygroscopicity, surface tension, viscosity and optical properties that can be gained from detailed laboratory measurements for complex mixtures through to surrogates for secondary organic atmospheric aerosols.

Original language	English
Pages (from-to)	639–661
Number of pages	23
Journal	Faraday Discuss.
Volume	200
Issue number	639
Early online date	27 Jan 2017
DOIs	https://doi.org/10.1039/C7FD00008A
Publication status	E-pub ahead of print - 27 Jan 2017

Bibliographical note

© Royal Society of Chemistry 2017. This is an author-produced version of the published paper. Uploaded in accordance with the publisher’s self-archiving policy. Further copying may not be permitted; contact the publisher for details.

Access to Document

10.1039/C7FD00008A

c7fd00008a
© Royal Society of Chemistry 2017. This is an author-produced version of the published paper. Uploaded in accordance with the publisher’s self-archiving policy. Further copying may not be permitted; contact the publisher for details.
Accepted author manuscript, 1.82 MB

Diffusion and Equilibration in Viscous Atmospheric Aerosol
Hamilton, J.
NATURAL ENVIRONMENT RESEARCH COUNCIL
2/02/15 → 1/02/18
Project: Research project (funded) › Research

Cite this

Marsh, A., Rovelli, G., Song, Y.-C., Pereira, K. L., Willoughby, R., Bzdek, B., Hamilton, J. F., Orr-Ewing, A., Topping, D., & Jonathan, R. (2017). Accurate Representations of the Physicochemical Properties of Atmospheric Aerosols: When are Laboratory Measurements of Value? Faraday Discuss., 200(639), 639–661. Advance online publication. https://doi.org/10.1039/C7FD00008A

@article{a06afd07bcf84dadabbfad1dbe46942a,

title = "Accurate Representations of the Physicochemical Properties of Atmospheric Aerosols:: When are Laboratory Measurements of Value?",

abstract = "Laboratory studies can provide important insights into the processes that occur at the mesoscale in ambient aerosol. We examine the accuracies of measurements of core physicochemical properties of aerosols that can be made in single particle studies and explore the impact of these properties on the microscopic processes that occur in ambient aerosol. Presenting new measurements, we examine here the refinements in our understanding of aerosol hygroscopicity, surface tension, viscosity and optical properties that can be gained from detailed laboratory measurements for complex mixtures through to surrogates for secondary organic atmospheric aerosols.",

author = "Aleksandra Marsh and Grazia Rovelli and Young-Chul Song and Pereira, {Kelly Louise} and Rose Willoughby and Bryan Bzdek and Hamilton, {Jacqueline Fiona} and andrew Orr-Ewing and David Topping and Reid Jonathan",

note = "{\textcopyright} Royal Society of Chemistry 2017. This is an author-produced version of the published paper. Uploaded in accordance with the publisher{\textquoteright}s self-archiving policy. Further copying may not be permitted; contact the publisher for details.",

year = "2017",

month = jan,

day = "27",

doi = "10.1039/C7FD00008A",

language = "English",

volume = "200",

pages = "639–661",

journal = "Faraday Discuss.",

publisher = "The Royal Society of Chemistry",

number = "639",

}

TY - JOUR

T1 - Accurate Representations of the Physicochemical Properties of Atmospheric Aerosols:

T2 - When are Laboratory Measurements of Value?

AU - Marsh, Aleksandra

AU - Rovelli, Grazia

AU - Song, Young-Chul

AU - Pereira, Kelly Louise

AU - Willoughby, Rose

AU - Bzdek, Bryan

AU - Hamilton, Jacqueline Fiona

AU - Orr-Ewing, andrew

AU - Topping, David

AU - Jonathan, Reid

N1 - © Royal Society of Chemistry 2017. This is an author-produced version of the published paper. Uploaded in accordance with the publisher’s self-archiving policy. Further copying may not be permitted; contact the publisher for details.

PY - 2017/1/27

Y1 - 2017/1/27

N2 - Laboratory studies can provide important insights into the processes that occur at the mesoscale in ambient aerosol. We examine the accuracies of measurements of core physicochemical properties of aerosols that can be made in single particle studies and explore the impact of these properties on the microscopic processes that occur in ambient aerosol. Presenting new measurements, we examine here the refinements in our understanding of aerosol hygroscopicity, surface tension, viscosity and optical properties that can be gained from detailed laboratory measurements for complex mixtures through to surrogates for secondary organic atmospheric aerosols.

AB - Laboratory studies can provide important insights into the processes that occur at the mesoscale in ambient aerosol. We examine the accuracies of measurements of core physicochemical properties of aerosols that can be made in single particle studies and explore the impact of these properties on the microscopic processes that occur in ambient aerosol. Presenting new measurements, we examine here the refinements in our understanding of aerosol hygroscopicity, surface tension, viscosity and optical properties that can be gained from detailed laboratory measurements for complex mixtures through to surrogates for secondary organic atmospheric aerosols.

U2 - 10.1039/C7FD00008A

DO - 10.1039/C7FD00008A

M3 - Article

VL - 200

SP - 639

EP - 661

JO - Faraday Discuss.

JF - Faraday Discuss.

IS - 639

ER -

Accurate Representations of the Physicochemical Properties of Atmospheric Aerosols: When are Laboratory Measurements of Value?

Abstract

Bibliographical note

Access to Document

Projects

Diffusion and Equilibration in Viscous Atmospheric Aerosol

Cite this