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An Expedient Protecting-Group-Free Total Synthesis of (±)-Dievodiamine

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Publication details

JournalOrganic Letters
DatePublished - 20 Jun 2013
Issue number13
Pages (from-to)3302-3305
Original languageEnglish


The first total synthesis of the Evodia rutaecarpa derived natural product dievodiamine is described. The convergent synthesis was performed without protecting groups, delivering a route that is short and high yielding and uses limited chromatography. Key steps include organometallic addition into a DHED adduct and the Stille coupling of two advanced intermediates to complete the synthesis.


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