Impact of the june 2018 saddleworth moor wildfires on air quality in Northern England

A. M. Graham*, R. J. Pope, J. B. McQuaid, K. P. Pringle, S. R. Arnold, A. G. Bruno, D. P. Moore, J. J. Harrison, M. P. Chipperfield, R. Rigby, A. Sanchez-Marroquin, J. Lee, S. Wilde, R. Siddans, B. J. Kerridge, L. J. Ventress, B. G. Latter

*Corresponding author for this work

Research output: Contribution to journalLetterpeer-review

Abstract

The June 2018 Saddleworth Moor fires were some of the largest UK wildfires on record and lasted for approximately three weeks. They emitted large quantities of smoke, trace gases and aerosols which were transported downwind over the highly populated regions of Manchester and Liverpool. Surface observations of PM2.5 indicate that concentrations were 4–5.5 times higher than the recent seasonal average. State-of-the-art satellite measurements of total column carbon monoxide (TCCO) from the TROPOMI instrument on the Sentinel 5—Precursor (S5P) platform, coupled with measurements from a flight of the UK BAe-146–301 research aircraft, are used to quantify the substantial enhancement in emitted trace gases. The aircraft measured plume enhancements with near-fire CO and PM2.5 concentrations >1500 ppbv and >125 μgm−3 (compared to ∼100 ppbv and ∼5 μgm−3 background concentrations). Downwind fire-plume ozone (O3) values were larger than the near-fire location, indicating O3 production with distance from source. The near-fire O3:CO ratio was (ΔO3/ΔCO) 0.001 ppbv/ppbv, increasing downwind to 0.060–0.105 ppbv/ppbv, suggestive of O3 production enhancement downwind of the fires. Emission rates of CO and CO2 ranged between 1.07 (0.07–4.69) kg s−1 and 13.7 (1.73–50.1) kg s−1, respectively, similar to values expected from a medium sized power station.

Original languageEnglish
Article number031001
JournalEnvironmental Research Communications
Volume2
Issue number3
DOIs
Publication statusPublished - 2020

Bibliographical note

Funding Information:
This work was supported by the UK Natural Environment Research Council (NERC) by providing funding for the National Centre for Earth Observation (NCEO) through grant number NE/R016518/1. The contribution of Alberto Sanchez-Marroquin has been supported by the European Research Council (MarineIce (grant no. 648661)). Surface pressure reanalysis charts from the UK Met Office were accessed from University of Leeds archive. Surface PM2.5 concentration observations were taken from the AURN network via https://uk-air.defra.gov.uk/ . The TROPOMI total column CO and tropospheric column NO2 data were obtained from ESA?s Copernicus Open Access Hub (https://scihub.copernicus.eu/) and the Tropospheric Emissions Monitoring Internet Service (TEMIS, http://temis.nl/airpollution/no2.html), respectively. MODIS fire radiative power (FRP) data was provided by the ECMWF Global Fire Assimilation System (https://apps.ecmwf.int/datasets/data/cams-gfas/). ECMWF ERA-Interim meteorological reanalysis data came from https://apps.ecmwf.int/datasets/ data/interim-full-daily/levtype=sfc/. The Saddleworth Moor aircraft data were taken using the Facility for Airborne Atmospheric Measurements (FAAM) BAe-146?301 Large Atmospheric Research Aircraft and are available from the Centre for Environmental Data Analysis (CEDA) at https://old.faam.ac.uk/index.php/data. The authors also gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (https://ready.noaa.gov) used in this publication.

Funding Information:
This work was supported by the UK Natural Environment Research Council (NERC) by providing funding for the National Centre for Earth Observation (NCEO) through grant number NE/R016518/1. The contribution of Alberto Sanchez-Marroquin has been supported by the European Research Council (MarineIce (grant no. 648661)). Surface pressure reanalysis charts from the UK Met Office were accessed from University of Leeds archive. Surface PM2.5 concentration observations were taken from the AURN network via https://uk-air.defra.gov.uk/ . The TROPOMI total column CO and tropospheric column NO2 data were obtained from ESA’s Copernicus Open Access Hub (https://scihub.copernicus.eu/) and the Tropospheric Emissions Monitoring Internet Service (TEMIS, http://temis.nl/airpollution/no2.html), respectively. MODIS fire radiative power (FRP) data was provided by the ECMWF Global Fire Assimilation System (https://apps.ecmwf.int/datasets/data/cams-gfas/). ECMWF ERA-Interim meteorological reanalysis data came from https://apps.ecmwf.int/datasets/ data/interim-full-daily/levtype=sfc/. The Saddleworth Moor aircraft data were taken using the Facility for Airborne Atmospheric Measurements (FAAM) BAe-146–301 Large Atmospheric Research Aircraft and are available from the Centre for Environmental Data Analysis (CEDA) at https://old.faam.ac.uk/index.php/data. The authors also gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (https://ready.noaa.gov) used in this publication.

Publisher Copyright:
© 2020 The Author(s). Published by IOP Publishing Ltd.

Keywords

  • Air quality
  • Aircraft observations
  • AURN
  • Earth observation
  • FAAM
  • TROPOMI
  • Wildfire

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