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Increasing Catalyst Efficiency in C−H Activation Catalysis

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JournalAngewandte Chemie - International Edition
DateAccepted/In press - 10 Nov 2017
DatePublished (current) - 23 Feb 2018
Issue number9
Volume57
Number of pages11
Pages (from-to)2296-2306
Original languageEnglish

Abstract

C−H activation reactions with high catalyst turnover numbers are still very rare in the literature and 10 mol % is a common catalyst loading in this field. We offer a representative overview of efficient C−H activation catalysis to highlight this neglected aspect of catalysis development and inspire future effort towards more efficient C−H activation. Examples ranging from palladium catalysis, Cp*Rh III - and Cp*Co III -catalysis, the C−H borylation and silylation to methane C−H activation are presented. In these reactions, up to tens of thousands of catalyst turnovers have been observed.

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© 2018 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim. This is an author-produced version of the published paper. Uploaded in accordance with the publisher’s self-archiving policy. Further copying may not be permitted; contact the publisher for details.

    Research areas

  • catalysis, C−H activation, methane, palladium, rhodium, turnover

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