Research output: Contribution to journal › Article › peer-review
Magnetic tunnel junctions with a B2-ordered CoFeCrAl equiatomic Heusler alloy. / Tsuchiya, Tomoki; Roy, Tufan; Elphick, Kelvin; Okabayashi, Jun; Bainsla, Lakhan; Ichinose, Tomohiro; Suzuki, Kazuya; Tsujikawa, Masahito; Shirai, Masafumi; Hirohata, Atsufumi; Mizukami, Shigemi.
In: PHYSICAL REVIEW MATERIALS, Vol. 3, No. 8, 084403, 05.08.2019.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Magnetic tunnel junctions with a B2-ordered CoFeCrAl equiatomic Heusler alloy
AU - Tsuchiya, Tomoki
AU - Roy, Tufan
AU - Elphick, Kelvin
AU - Okabayashi, Jun
AU - Bainsla, Lakhan
AU - Ichinose, Tomohiro
AU - Suzuki, Kazuya
AU - Tsujikawa, Masahito
AU - Shirai, Masafumi
AU - Hirohata, Atsufumi
AU - Mizukami, Shigemi
N1 - © 2019 American Physical Society. This is an author-produced version of the published paper. Uploaded in accordance with the publisher’s self-archiving policy. Further copying may not be permitted; contact the publisher for details.
PY - 2019/8/5
Y1 - 2019/8/5
N2 - The equiatomic quaternary Heusler alloy CoFeCrAl is a candidate material for spin-gapless semiconductors (SGSs). However, to date, there have been no experimental attempts at fabricating a junction device. This paper reports a fully epitaxial (001)-oriented MgO barrier magnetic tunnel junction (MTJ) with CoFeCrAl electrodes grown on a Cr buffer. X-ray and electron diffraction measurements show that the (001) CoFeCrAl electrode films with atomically flat surfaces have a B2-ordered phase. The saturation magnetization is 380 emu/cm3, almost the same as the value given by the Slater–Pauling–like rule, and the maximum tunnel magnetoresistance ratios at 300 K and 10 K are 87% and 165%, respectively. Cross-sectional electron diffraction analysis shows that the MTJs have MgO interfaces with fewer dislocations. The temperature- and bias-voltage dependence of the transport measurements indicates magnon-induced inelastic electron tunneling overlapping with the coherent electron tunneling. X-ray magnetic circular dichroism (XMCD) measurements show a ferromagnetic arrangement of the Co and Fe magnetic moments of B2-ordered CoFeCrAl, in contrast to the ferrimagnetic arrangement predicted for the Y -ordered state possessing SGS characteristics. Ab-initio calculations taking account of the Cr-Fe swap disorder qualitatively explain the XMCD results. Finally, the effect of the Cr-Fe swap disorder on the ability for electronic states to allow coherent electron tunneling is discussed.
AB - The equiatomic quaternary Heusler alloy CoFeCrAl is a candidate material for spin-gapless semiconductors (SGSs). However, to date, there have been no experimental attempts at fabricating a junction device. This paper reports a fully epitaxial (001)-oriented MgO barrier magnetic tunnel junction (MTJ) with CoFeCrAl electrodes grown on a Cr buffer. X-ray and electron diffraction measurements show that the (001) CoFeCrAl electrode films with atomically flat surfaces have a B2-ordered phase. The saturation magnetization is 380 emu/cm3, almost the same as the value given by the Slater–Pauling–like rule, and the maximum tunnel magnetoresistance ratios at 300 K and 10 K are 87% and 165%, respectively. Cross-sectional electron diffraction analysis shows that the MTJs have MgO interfaces with fewer dislocations. The temperature- and bias-voltage dependence of the transport measurements indicates magnon-induced inelastic electron tunneling overlapping with the coherent electron tunneling. X-ray magnetic circular dichroism (XMCD) measurements show a ferromagnetic arrangement of the Co and Fe magnetic moments of B2-ordered CoFeCrAl, in contrast to the ferrimagnetic arrangement predicted for the Y -ordered state possessing SGS characteristics. Ab-initio calculations taking account of the Cr-Fe swap disorder qualitatively explain the XMCD results. Finally, the effect of the Cr-Fe swap disorder on the ability for electronic states to allow coherent electron tunneling is discussed.
U2 - 10.1103/PhysRevMaterials.3.084403
DO - 10.1103/PhysRevMaterials.3.084403
M3 - Article
VL - 3
JO - PHYSICAL REVIEW MATERIALS
JF - PHYSICAL REVIEW MATERIALS
SN - 2475-9953
IS - 8
M1 - 084403
ER -