Research output: Contribution to journal › Article › peer-review
Journal | ACS Sustainable Chemistry and Engineering |
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Date | Accepted/In press - 11 Jun 2018 |
Date | E-pub ahead of print - 11 Jun 2018 |
Date | Published (current) - 6 Aug 2018 |
Issue number | 8 |
Volume | 6 |
Number of pages | 9 |
Pages (from-to) | 9744-9752 |
Early online date | 11/06/18 |
Original language | English |
Ring-opening metathesis polymerization (ROMP) of biobased oxanorbornene amides by Grubbs second generation catalyst was used to prepare a range of well-defined homo- and copolymers. A series of 11 amide monomers, featuring a variety of functionalities including amino acids and peptides, have been synthesized from a biobased oxanorbornene acid, prepared through the 100% atom economical tandem Diels-Alder lactonization between itaconic anhydride and furfuryl alcohol. The polymerization has been shown to be well-controlled, with the prepared homo- and copolymers possessing controlled molecular weights with narrow polydispersities.
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