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Selective synthesis of three product classes from imine and carboxylic acid precursors via direct imine acylation

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JournalOrganic and Biomolecular Chemistry
DateAccepted/In press - 29 Aug 2017
DatePublished (current) - 5 Sep 2017
Volume15
Number of pages6
Pages (from-to)7527-7532
Original languageEnglish

Abstract

Three divergent Direct Imine Acylation (DIA) procedures are reported that allow the selective generation of δ-lactams, β-lactams and tetrahydropyrimidinones (via a novel three-component coupling) from imine and carboxylic acid precursors. All operate via initial N-acyliminium ion formation and diverge depending on the reaction conditions and nature of the substrates.

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© The Royal Society of Chemistry 2017. This is an author-produced version of the published paper. Uploaded in accordance with the publisher’s self-archiving policy. Further copying may not be permitted; contact the publisher for details

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