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The First Syntheses of (+/-)-SDEF 678 Metabolite and (+/-)-Speciosins A-C

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Publication details

JournalEuropean Journal of Organic Chemistry
DatePublished - Jan 2011
Issue number3
Number of pages4
Pages (from-to)451-454
Original languageEnglish

Abstract

The epoxyquinone natural products SDEF 678 metabolite, speciosin A, speciosin B and speciosin C have been prepared for the first time via a short synthetic route based around the palladium-catalysed coupling of a halogen-substituted 1,4-benzoquinone monoketal, a Diels-Alder/retro-Diels-Alder sequence and a diastereoselective epoxidation process.

    Research areas

  • Natural products, Quinones, Speciosins, COUPLING REACTIONS, MANUMYCIN FAMILY, ANTIBIOTICS, MONOKETALS, CATALYSIS, OXIDATION, EFFICIENT, ANALOGS, ROUTE

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