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Tributyltin hydride-mediated tandem reactions of dehydroalanines leading to alpha-substituted pyroglutamates

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Publication details

JournalJOURNAL OF CHEMICAL RESEARCH-S
DatePublished - Jul 2000
Issue number7
Number of pages2
Pages (from-to)312-313
Original languageEnglish

Abstract

Tributyltin hydride-mediated cyclisation of dehydroalanines produces an intermediate captodative radical, which can be trapped by reaction with oxygen- or carbon-centred radicals or (principally) electron-poor alkenes, to provide a quick approach to a variety of alpha-substituted pyroglutamates.

    Research areas

  • RADICAL CYCLIZATION, SECONDARY AMIDES, PYRROLIDINONES, 5-ENDO-TRIG, 4-EXO-TRIG

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